Chemical Sciences: A Manual for CSIR-UGC National Eligibility Test for Lectureship and JRF/RFQ Beam Coolers

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Despite its long history, high-sensitivity high-accuracy mass measurements of atomic nuclei continue to be very important areas of research for many branches of physics. Not only do these measurements provide us with a better understanding of nuclear structures and nuclear forces but they also offer insight into how matter behaves in some of Nature’s harshest environments. At facilities such as ISOLDE at CERN and TRIUMF in Vancouver, for instance, measurement techniques are now being extended to short-lived radionuclei that only occur naturally in the interior of exploding stars. Their short half-lives and very low production rates at even the most powerful facilities require the very highest in sensitivity of such measurements.

Penning traps, the central element in modern high-accuracy high-sensitivity mass measurement installations, enable measurements of accuracies approaching 1 part in 10^11 on single ions. However, to achieve this Penning traps must have the ion to be measured delivered to it very precisely and with certainty that it is indeed the desired ion. This imposes severe requirements on the apparatus that must take the atomic nucleus out of the target in which it has been created, sort it from the myriad of other ions that are emitted from the target and then direct it so that it can be captured in the measurement trap.

Cooling these ion beams, particularly radioactive ion beams, has been shown to drastically improve the accuracy and sensitivity of mass measurements by reducing the phase space of the ion collections in question. Using a light neutral background gas, typically helium, charged particles originating from on-line mass separators undergo a number of soft collisions with the background gas molecules resulting in fractional losses of the ions’ kinetic energy and a reduction of the ion ensemble’s overall energy. In order for this to be effective however, the ions need to be contained using transverse radiofrequency quadrupole (RFQ) electric fields during the collisional cooling process (also known as buffer gas cooling). These RFQ coolers operate on the same principles as quadrupole ion traps and have been shown to be particularly well suited for buffer gas cooling given their capacity for total confinement of ions having a large dispersion of velocities, corresponding to kinetic energies up to tens of electron volts. A number of the RFQ coolers have already been installed at research facilities around the world and a list of their characteristics can be found below.




RFQ Coolers Around the World
Name Input Beam Input Emittance Cooler Length R0 RF Voltage, Freq, DC Mass Range Axial Voltage Pressure Output Beam Qualities Images
Colette[1]

[2]

60 keV ISOLDE beam decelerated to ≤ 10 eV ~ 30 π-mm-mrad 504 mm (15 segments, electrically isolated) 7 mm Freq : 450 – 700 kHz -- 0.25 V/cm 0.01 mbar He Reaccelerated to up to 59.99 keV with long. energy spread ~10 eV COLETTE1

COLETTE2

LPC Cooler[3] SPIRAL type beams Up to ~ 100 π-mm-mrad 468 mm (26 segments, electrically isolated) 15 mm RF : up to 250 Vp, Freq : 500 kHz – 2.2 MHz -- -- up to 0.1 mbar -- LPC1

LPC2

SHIPTRAP Cooler[4]

[5] [6]

SHIP type beams 20-500 keV/A -- 1140 mm (29 segments, electrically isolated) 3.9 mm RF: 30-200 Vpp, Freq: 800 kHz – 1.2 MHz up to 260 amu Variable: 0.25 – 1 V/cm ~ 5×10-3 mbar He -- SHIPTRAP1

SHIPTRAP2

JYFL Cooler[7]

[8]

IGISOL type beam at 40 keV Up to 17 π-mm-mrad 400 mm (16 segmentes) 10 mm RF: 200 Vp, Freq: 300 kHz – 800 kHz -- ~1 V/cm ~0.1 mbar He ~3 π-mm-mrad, Energy spread < 4 eV JYFL1

JYFL2

JYFL3

MAFF Cooler[9] 30 keV beam decelerated to ~100 eV -- 450mm 30mm RF: 100 –150 Vpp, Freq: 5 MHz -- ~0.5 V/cm ~0.1 mbar He energy spread = 5 eV, Emittance @ 30keV: from = 36 π-mm-mrad to eT = 6 π-mm-mrad --
ORNL Cooler[10] 20-60 keV negative RIBs decelerated to <100 eV ~50 π-mm-mrad (@ 20 keV) 400 mm 3.5 mm RF: ~400 Vp, Freq: up to 2.7 MHz -- up to ±5 kV on tapered rods ~0.01 mbar Energy spread ~2 eV ORNL1

ORNL2

ORNL3

LEBIT Cooler[11] 5 keV DC beams -- -- -- -- -- -- ~1×x10−1 mbar He (high-pressure section) -- LEBIT1

LEBIT2

LEBIT3

ISCOOL[12]

[13]

60 keV ISOLDE beam up to 20 π-mm-mrad 800 mm (using segmented DC wedge electrodes) 20 mm RF: up to 380 V, Freq: 300 kHz - 3MHz 10-300 amu ~0.1V/cm 0,01 - 0,1 mbar He -- ISCOOL1

ISCOOL2

ISCOOL3

ISCOOL4

ISOLTRAP Cooler[14] 60 keV ISOLDE beam -- 860 mm (segmented) 6 mm RF: ~125 Vp, Freq: ~1 MHz. -- -- ~2×10-2 mbar He elong ≈ 10 eV us, etrans ≈ 10p mm mrad. ISOLTRAP1

ISOLTRAP2

TITAN RFCT[15] continuous 30–60 keV ISAC beam -- -- -- RF: 1000 Vpp, Freq: 300 kHz - 3 MHz -- -- -- 6 π-mm-mrad at 5 keV extraction energy TITAN1

TITAN2

TITAN3

TRIMP Cooler[16] TRIMP beams -- 660 mm (segmented) 5 mm RF= 100 Vp, Freq.: up to 1.5 MHz 6 < A < 250 -- up to 0.1 mbar -- TRIMP1

TRIMP2

TRIMP3

SPIG Leuven -- -- 124 mm (sextuple rod structure) 1.5 mm RF= 0-500 Vpp, Freq.: 4.7 MHz -- -- -- -- --
Argonne CPT -- -- -- -- -- -- -- -- -- --
SLOWRI cooler -- -- 600 mm (segmented sextuple rod structure) 8 mm RF= 400 Vpp, Freq.: 3.6 MHz -- -- ~10 mbar He -- --
-- -- -- -- -- -- -- -- -- -- --


References[edit]

  1. M. Sewtz, C. Bachelet, N. Chauvin, C. Guénaut, E. Leccia, D. Le Du and D. Lunney (2005). "Deceleration and cooling of heavy ion beams: The COLETTE project". Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms 240 (p. 55-60). 
  2. Cyril Bachelet (2004). Mesure de Masse de Noyaux à Halo et Refroidissement de Faisceaux avec l'Expérience Mistral. PhD Thesis. Université Paris XI, France. 
  3. Guillaume Darius (2004). Etude et Mise en oeuvre d'un Dispositif pour la Mesure de Paramètre de Correlation Angulaire dans la Désintégration du Noyau Hélium 6. PhD Thesis. Université de Caen / Basse-Normandie, France. 
  4. S. Rahaman, M. Block, D. Ackermann, D. Beck, A. Chaudhuri, S. Eliseev, H. Geissel, D. Habs, F. Herfurth, F.P. Heßberger et al. (2006). "On-line commissioning of SHIPTRAP". International Journal of Mass Spectrometry 251 (p. 146-151). 
  5. Jens Dilling (2001). Direct Mass Measurments on Exotic Nuclei with SHIPTRAP and ISOLTRAP. PhD Thesis. University of Heidelberg, Germany. 
  6. Daniel Rodriguez Rubiales (2001). An RFQ Buncher for Accumulation and Cooling of Heavy Radionuclides at SHIPTRAP and High Precision Mass Measurements on Unstable Kr Isotopes at ISOLTRAP. PhD Thesis. University of Valencia, Spain. 
  7. A. Jokinen, J. Huikari, A. Nieminen and J. Äystö (2002). "The first cooled beams from JYFL ion cooler and trap project". Nuclear Physics A 701 (p. 557-560). 
  8. Arto Nieminen (2002). Manipulation of Low-Energy Radioactive Ion Beams With an RFQ Cooler; Applications to Collinear Laser Spectroscopy. PhD Thesis. University of Jyväskylä, Jyväskylä, Finland. 
  9. J. Szerypo, D. Habs, S. Heinz, J. Neumayr, P. Thirolf, A. Wilfart and F. Voit (2003). "MAFFTRAP: ion trap system for MAFF". Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms 204 (p. 512-516). 
  10. Y. Liu, J.F. Liang G.D. Alton, J.R. Beene, Z. Zhou, H. Wollnik (2002). "Collisional Cooling of Negative-Ion Beams". Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms 187 (p. 117-131). 
  11. G. Bollen, S. Schwarz, D. Davies, P. Lofy, D. Morrissey, R. Ringle, P. Schury,T. Sun, L. Weissman (2004). "Beam cooling at the low-energy-beam and ion-trap facility at NSCL/MSU". Nuclear Instruments and Methods in Physics Research A 532 (p. 203–209). 
  12. I. Podadera Aliseda, T. Fritioff, T. Giles, A. Jokinen, M. Lindroos and F. Wenander (2004). "Design of a second generation RFQ Ion Cooler and Buncher (RFQCB) for ISOLDE". Nuclear Physics A 746 (p. 647-650). 
  13. Ivan Podadera Aliseda (2006). New Developments on Preparation of Cooled and Bunched Radioactive Ion Beams at ISOL-Facilities: The ISCOOL Project and Rotating-Wall Cooling. PhD Thesis. CERN, Geneva, Switzerland. 
  14. T. J. Giles, R. Catherall, V. Fedosseev, U. Georg, E. Kugler, J. Lettry and M. Lindroos (2003). "The high resolution spectrometer at ISOLDE". Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms 204 (p. 497-501). 
  15. J. Dilling, P. Bricault, M. Smith, H. -J. Kluge and TITAN collaboration (2003). "The proposed TITAN facility at ISAC for very precise mass measurements on highly charged short-lived isotopes". Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms 204 (Pages 492-496). 
  16. Emil Traykov (2006). Production of Radioactive Beams for Atomic Trapping. PhD Thesis. University of Groningen, The Netherlands. 

Further Reading[edit]

  • SHIPTRAP collaboration, J. Schönfelder, D. Ackermann, H. Backe, G. Bollen, J. Dilling, A. Dretzke, O. Engels, J. Estermann, D. Habs, S. Hofmann, F. P. Hessberger, H. -J. Kluge, W. Lauth, W. Ludolphs, M. Maier, G. Marx, R. B. Moore, W. Quint, D. Rodriguez, M. Sewtz, G. Sikler, C. Toader and Chr. Weber (2002). "SHIPTRAP—a capture and storage facility for heavy radionuclides at GSI". Nuclear Physics A 701 (p. 579-582). 
  • G. Sikler, D. Ackermann, F. Attallah, D. Beck, J. Dilling, S. A. Elisseev, H. Geissel, D. Habs, S. Heinz, F. Herfurth et al. (2003). "First on-line test of SHIPTRAP". Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms 204 (p. 482-486). 
  • J.B. Neumayr, L. Beck, D. Habs, S. Heinz, J. Szerypo, P.G. Thirolf, V. Varentsov, F. Voit, D. Ackermann, D. Beck et al. (2006). "The ion-catcher device for SHIPTRAP". Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms 244 (p. 489-500). 
  • J. Szerypo, A. Jokinen, V. S. Kolhinen, A. Nieminen, S. Rinta-Antila and J. Äystö (2002). "Penning trap at IGISOL". Nuclear Physics A 701 (p. 588-591). 
  • T. Faestermann, W. Assmann, L. Beck, H. Bongers, W. Carli, M. Groß, R. Großmann, D. Habs, P. Hartung, S. Heinz et al. (2004). "The Munich Accelerator for Fission Fragments - MAFF". Nuclear Physics A 746 (p. 22-26). 
  • D. Habs, M. Groß, W. Assmann, F. Ames, H. Bongers, S. Emhofer, S. Heinz, S. Henry, O. Kester, J. Neumayr et al. (2003). "The Munich accelerator for fission fragments MAFF". Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms 204 (p. 739-745). 
  • F. Herfurth, J. Dilling, A. Kellerbauer, G. Bollen, S. Henry, H. -J. Kluge, E. Lamour, D. Lunney, R. B. Moore, C. Scheidenberger et al. (2001). "A linear radiofrequency ion trap for accumulation, bunching, and emittance improvement of radioactive ion beams". Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment 469 (p. 254-275). 
  • S. Schwarz, G. Bollen, D. Lawton, A. Neudert, R. Ringle, P. Schury and T. Sun (2003). "A second-generation ion beam buncher and cooler". Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms 204 (p. 474-477). 
  • J. Clark, R. C. Barber, C. Boudreau, F. Buchinger, J. E. Crawford, S. Gulick, J. C. Hardy, A. Heinz, J. K. P. Lee, R. B. Moore et al. (2003). "Improvements in the injection system of the Canadian Penning trap mass spectrometer". Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms 204 (p. 487-491).